Abstract Herein, we report the synthesis and characterization of chrysoidine (4-phenylazo-m-phenylenediamine) grafted on magnetic nanoparticles ( Fe3O4@SiO2@CPTMS@PhAzPhDA = FeSiPAPDA) as a novel and versatile adsorbent used for the satisfactory removal of Pb, Ni, and Cd ions from contaminated water via the formation of their complexes. The Freundlich, Langmuir, Temkin, and Redlich-Patterson isotherm models were studied to reveal the adsorption capability of the adsorbent and were found out that the Langmuir model is more compatible with the nano-adsorbent behavior. Moreover, according to the ICP tests as well as based on the Langmuir isotherm, the maximum adsorption capacity
