Due to the environmental pollution issues and the supply of drinking/clean water, removal of both inorganic and organic (particularly dyes, nitroarenes, and heavy metals) to non-dangerous products and useful compounds are very important transformations. The deployment of sustainable and eco-friendly nanomaterials with exceptional structural and unique features such as high efficiency and stability/recyclability, high surface/volume ratio, low- cost production routes has become a priority; nonetheless, numerous significant challenges/restrictions still remained unresolved. The immobilization of green synthesized metal nanoparticles (NPs) on the natural mate- rials and biowaste generated templates have been analyzed widely as a greener approach due to their envi- ronmentally friendly preparation methods, earth-abundance, cost-effectiveness with low energy consumption, biocompatibility, as well as adjustability in various cases of biomolecules as bioreducing agents. Natural and biowaste materials are widely considered as important sources to fabricate greener and biosynthesized types of metal, metal oxide, and metal sulfide nanomaterials using plant extracts. Integrating green synthesized nano- particles with various biotemplates offers new practical composites for mitigating environmental challenges. In this review, degradation of dyes, reduction of toxic nitrophenols, absorption of heavy metals, and other haz- ardous/toxic environmental pollutants from contaminated water bodies using biowaste- and nature-derived nanomaterials are highlighted.